Not yet. For now if your libcall selection depends on a subtarget feature, you still need to manually configure it (by the enum value) in the TargetLowering constructor. The target’s SystemRuntimeLibrary should include the superset of calls that any subtarget could use.
I’m working on moving the codegen component into tablegen. In the future there should be a separate LibcallLoweringInfo corresponding to the current TargetLowering table, separate from the triple’s list of libcalls